This site has TONS of resources for structured play, beginning literacy activities, and hand-eye coordination broken down by age from birth and through school years. Stoplight Beanbag Toss - I Can Teach My Child! I own bean bags already!
Easy and fun.Velcro + popsicle sticks make for great quiet time or restaurant activity. Put velcro dots on the ends of popsicle sticks. Kids can make letters or shapes over and over again. I found velcro dots at my local dollar store.